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Issue 53, 2020
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Synergetic effect of H+ adsorption and ethylene functional groups of covalent organic frameworks on the CO2 photoreduction in aqueous solution

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Abstract

We prepare a novel COF for CO2 photoreduction with 99.9% CO selectivity in aqueous solution without a cocatalyst. DFT shows that the preferential adsorption of H+ on the COF results in increased CO2 adsorption energy providing an anchoring site of CO2, and with the cooperation of an ethylene group, CO2 reduction is triggered.

Graphical abstract: Synergetic effect of H+ adsorption and ethylene functional groups of covalent organic frameworks on the CO2 photoreduction in aqueous solution

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Article information


Submitted
22 Apr 2020
Accepted
20 May 2020
First published
24 May 2020

Chem. Commun., 2020,56, 7261-7264
Article type
Communication

Synergetic effect of H+ adsorption and ethylene functional groups of covalent organic frameworks on the CO2 photoreduction in aqueous solution

J. Zhou, J. Cui, M. Dong, C. Sun, S. You, X. Wang, Z. Zhou and Z. Su, Chem. Commun., 2020, 56, 7261
DOI: 10.1039/D0CC02896G

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