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Highly dispersed nickel anchored on a N-doped carbon molecular sieve derived from metal–organic frameworks for efficient hydrodeoxygenation in the aqueous phase

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Abstract

ZIF-8 was employed as a template to synthesize HD-Ni/N-CMS containing highly dispersed Ni at the atomic level anchored on a N-doped carbon molecular sieve for vanillin hydrodeoxygenation. The ZIF-8 structure was inherited and NiN bonds were formed by the coordination of Ni with N-rich defects, therefore it exhibited a high turnover frequency (1047.1 h−1) and good stability.

Graphical abstract: Highly dispersed nickel anchored on a N-doped carbon molecular sieve derived from metal–organic frameworks for efficient hydrodeoxygenation in the aqueous phase

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Article information


Submitted
11 Apr 2020
Accepted
06 May 2020
First published
06 May 2020

Chem. Commun., 2020, Advance Article
Article type
Communication

Highly dispersed nickel anchored on a N-doped carbon molecular sieve derived from metal–organic frameworks for efficient hydrodeoxygenation in the aqueous phase

R. Fan, Z. Hu, C. Chen, X. Zhu, H. Zhang, Y. Zhang, H. Zhao and G. Wang, Chem. Commun., 2020, Advance Article , DOI: 10.1039/D0CC02620D

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