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Metal cation-exchanged zeolites with the location, state, and size of metal species controlled

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Abstract

Rh ion-exchanged MFI-type aluminosilicate zeolites with different Al distributions were prepared for controlling the location, state, and size of Rh species. The MFI-type aluminosilicate zeolite with the framework Al atoms predominantly located inside the channel intersections leads to the formation of relatively large Rh species, which were confirmed by ultraviolet-visible (UV-vis) and infrared (IR) spectroscopies. Moreover, this catalyst showed a high catalytic activity for the oxidative reforming reaction of methane.

Graphical abstract: Metal cation-exchanged zeolites with the location, state, and size of metal species controlled

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Article information


Submitted
29 Mar 2020
Accepted
21 Apr 2020
First published
21 Apr 2020

Chem. Commun., 2020, Advance Article
Article type
Communication

Metal cation-exchanged zeolites with the location, state, and size of metal species controlled

R. Osuga, S. Bayarsaikhan, S. Yasuda, R. Manabe, H. Shima, S. Tsutsuminai, A. Fukuoka, H. Kobayashi and T. Yokoi, Chem. Commun., 2020, Advance Article , DOI: 10.1039/D0CC02284E

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