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ArNMeCH(SiMe3)2: a useful precursor of formal α-aminoalkyl diradicals in visible-light-mediated homo- and hetero-diaddition with alkenes

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Abstract

ArNMeCH(SiMe3)2 has been developed as a useful precursor of a formal α-aminoalkyl diradical in Ru(bpy)3Cl2-catalzyed addition with alkenes under visible-light-mediated photoredox conditions. This approach leads to homo-diaddition with two identical alkenes in one-pot, or hetero-diaddition with two different alkenes via a sequential operation.

Graphical abstract: ArNMeCH(SiMe3)2: a useful precursor of formal α-aminoalkyl diradicals in visible-light-mediated homo- and hetero-diaddition with alkenes

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Article information


Submitted
28 Mar 2020
Accepted
22 May 2020
First published
25 May 2020

Chem. Commun., 2020, Advance Article
Article type
Communication

ArNMeCH(SiMe3)2: a useful precursor of formal α-aminoalkyl diradicals in visible-light-mediated homo- and hetero-diaddition with alkenes

S. Liu, Y. Yang, L. Gao and Z. Song, Chem. Commun., 2020, Advance Article , DOI: 10.1039/D0CC02277B

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