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Issue 92, 2020
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Nickel(ii)-modified covalent-organic framework film for electrocatalytic oxidation of 5-hydroxymethylfurfural (HMF)

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Abstract

Electrochemical oxidation of 5-hydroxymethylfurfural (HMF) is a promising synthetic route for 2,5-furandicarboxylic acid (FDCA) production. Here, we prepared a nickel(II)-modified covalent-organic framework (COF) film TpBpy-Ni@FTO for HMF electrooxidation. With a high conversion of HMF (96%), TpBpy-Ni@FTO afforded a 58% FDCA yield. This work underlines the great potential of COF-based materials in electrocatalysis.

Graphical abstract: Nickel(ii)-modified covalent-organic framework film for electrocatalytic oxidation of 5-hydroxymethylfurfural (HMF)

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Article information


Submitted
25 Mar 2020
Accepted
22 Oct 2020
First published
22 Oct 2020

Chem. Commun., 2020,56, 14361-14364
Article type
Communication

Nickel(II)-modified covalent-organic framework film for electrocatalytic oxidation of 5-hydroxymethylfurfural (HMF)

M. Cai, S. Ding, B. Gibbons, X. Yang, M. C. Kessinger and A. J. Morris, Chem. Commun., 2020, 56, 14361
DOI: 10.1039/D0CC02206C

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