Issue 47, 2020
From the journal:

Chemical Communications

Unravelling the role of active-site isolation in reactivity and reaction pathway control for acetylene hydrogenation†

Siyang Liu,‡ab   Yiming Niu,‡bc   Yongzhao Wang,bc   Junnan Chen,bc   Xueping Quan,b   Xia Zhang ORCID logo *a  and  Bingsen Zhang ORCID logo *bcd  

* Corresponding authors

a Department of Chemistry, College of Science, Northeastern University, Shenyang 110819, China
E-mail: xzhang@mail.neu.edu.cn

b Shenyang National Laboratory for Materials Science, Institute of Metal Research, Chinese Academy of Sciences, Shenyang 110016, China
E-mail: bszhang@imr.ac.cn

c School of Materials Science and Engineering, University of Science and Technology of China, Shenyang 110016, China

d Dalian National Laboratory for Clean Energy, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian 116023, China

Abstract

Supported bimetallic PdxCuy catalysts with precisely controlled Pd/Cu ratios were prepared and characterized by combining sample averaged and microscopic techniques. The active-site isolation effect on reactivity and reaction pathway control with different extent of Pd ensembles in acetylene hydrogenation is unravelled systematically.

Graphical abstract: Unravelling the role of active-site isolation in reactivity and reaction pathway control for acetylene hydrogenation

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Article information

DOI
https://doi.org/10.1039/D0CC01889A
Article type
Communication
Submitted
12 Mar 2020
Accepted
26 Apr 2020
First published
27 Apr 2020

Chem. Commun., 2020,56, 6372-6375

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Unravelling the role of active-site isolation in reactivity and reaction pathway control for acetylene hydrogenation

S. Liu, Y. Niu, Y. Wang, J. Chen, X. Quan, X. Zhang and B. Zhang, Chem. Commun., 2020, 56, 6372 DOI: 10.1039/D0CC01889A

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