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Boosting efficient ambient nitrogen oxidation by a well-dispersed Pd on MXene electrocatalyst

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Abstract

An electrochemical nitrogen oxidation approach has been realized experimentally by a Pd-decorated MXene (Ti3C2Tx, T = F and O) electrocatalyst under ambient conditions. The Pd-MXene catalyst can achieve a desirable nitrate yield rate of 2.80 μg h−1 mgcat−1 (equivalent to 45.16 μmol h−1 gcat−1 HNO3) as well as a high nitrate faradaic efficiency of 11.34% in a favorable neutral pH environment.

Graphical abstract: Boosting efficient ambient nitrogen oxidation by a well-dispersed Pd on MXene electrocatalyst

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Article information


Submitted
06 Mar 2020
Accepted
15 Apr 2020
First published
15 Apr 2020

Chem. Commun., 2020, Advance Article
Article type
Communication

Boosting efficient ambient nitrogen oxidation by a well-dispersed Pd on MXene electrocatalyst

W. Fang, C. Du, M. Kuang, M. Chen, W. Huang, H. Ren, J. Xu, A. Feldhoff and Q. Yan, Chem. Commun., 2020, Advance Article , DOI: 10.1039/D0CC01759K

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