We have adapted solid phase phosphoramidite synthesis commonly used to make DNA, to produce two sequence-isomeric non-biological polymers which display sequence-programmed folding and self-assembly, going beyond structures which would be trivially anticipated. These findings open up possibilities for more sophisticated sequence/structure relationships using the same synthetic platform.
N. Appukutti, J. R. Jones and C. J. Serpell, Chem. Commun., 2020, 56, 5307 DOI: 10.1039/D0CC01319F
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