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Palladium-catalyzed intermolecular C–H silylation initiated by aminopalladation

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Abstract

A Pd(II)-catalyzed intermolecular C–H silylation reaction initiated by aminopalladation has been developed. The C–H bonds were activated by an alkyl Pd(II) species generated through aminopalladation and then disilylated with hexamethyldisilane to form disilylated indolines as the final products. The reaction provides a new method for the introduction of silyl groups into complex organic molecules.

Graphical abstract: Palladium-catalyzed intermolecular C–H silylation initiated by aminopalladation

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Article information


Submitted
03 Feb 2020
Accepted
09 Jun 2020
First published
09 Jun 2020

Chem. Commun., 2020, Advance Article
Article type
Communication

Palladium-catalyzed intermolecular C–H silylation initiated by aminopalladation

X. Ji, F. Wei, B. Wan, C. Cheng and Y. Zhang, Chem. Commun., 2020, Advance Article , DOI: 10.1039/D0CC00872A

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