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Transformation of a proton insulator to a conductor via reversible amorphous to crystalline structure transformation of MOFs

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Abstract

In this study, a successful proton conduction modulation of MOFs, from an ionic insulator to an ionic conductor, is demonstrated through their structural transformation. It is shown that the reversible structural change from amorphous to crystalline phases allows for the reversible proton conduction modulation of MOFs. Moreover, the proton conduction mechanism of the ionic conductor phase is elucidated by 2H NMR analysis.

Graphical abstract: Transformation of a proton insulator to a conductor via reversible amorphous to crystalline structure transformation of MOFs

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Article information


Submitted
29 Jan 2020
Accepted
06 Mar 2020
First published
09 Mar 2020

Chem. Commun., 2020, Advance Article
Article type
Communication

Transformation of a proton insulator to a conductor via reversible amorphous to crystalline structure transformation of MOFs

Y. Song, A. E. Khudozhitkov, J. Lee, H. Kang, D. I. Kolokolov, A. G. Stepanov and M. Yoon, Chem. Commun., 2020, Advance Article , DOI: 10.1039/D0CC00755B

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