A new bis-hydroxyphenylpyrazolyl ligand, H4L, allows isolating and structurally characterizing vanadyl and titanyl dinuclear complexes (Bu4N)2[(MO)2(HL)2] (M = V, Ti). The weak dipolar coupling and relatively short quantum coherence of the divanadyl anions are optimal for a 2-qubit molecular architecture proposed to implement electron-mediated nuclear quantum simulations.
I. Borilovic, P. J. Alonso, O. Roubeau and G. Aromí, Chem. Commun., 2020, 56, 3139 DOI: 10.1039/C9CC09817H
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