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Nickel-catalyzed regio- and diastereoselective hydroarylative and hydroalkenylative cyclization of 1,6-dienes

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Abstract

An unprecedented nickel-catalyzed hydroarylative and hydroalkenylative cyclization of unsymmetrically substituted 1,6-dienes with organoboronic acid was developed by using MeOH as the hydrogen source and employing commercially available Ni(η2-1,5-cyclooctadiene)2 as the catalyst. A series of biologically interesting cyclic products were afforded in moderate to excellent yields with high regio- and diastereoselectivities.

Graphical abstract: Nickel-catalyzed regio- and diastereoselective hydroarylative and hydroalkenylative cyclization of 1,6-dienes

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Article information


Submitted
05 Dec 2019
Accepted
29 May 2020
First published
29 May 2020

Chem. Commun., 2020, Advance Article
Article type
Communication

Nickel-catalyzed regio- and diastereoselective hydroarylative and hydroalkenylative cyclization of 1,6-dienes

Z. Xu, Y. Tang, C. Shen, H. Zhang, Y. Gan, X. Ji, X. Tian and K. Dong, Chem. Commun., 2020, Advance Article , DOI: 10.1039/C9CC09450D

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