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Temperature-responsive dissolution/recrystallization of Zn MOF enables the maximum efficiency and recyclability of catalysts

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Abstract

A novel strategy through a temperature-responsive dissolution and recrystallization process has successfully achieved 100% atomic utilization and easy recyclability of heterogeneous metal organic framework dimethylammonium zinc formate (DMZnF) catalysts for highly efficient dehydrogenation of DMF–H2O for hydrogen generation. DMZnF dissolves as a homogeneous catalyst at high reaction temperatures and then is recrystallized and recycled as a heterogeneous catalyst at low temperatures.

Graphical abstract: Temperature-responsive dissolution/recrystallization of Zn MOF enables the maximum efficiency and recyclability of catalysts

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Article information


Submitted
01 Dec 2019
Accepted
08 Jan 2020
First published
10 Jan 2020

Chem. Commun., 2020, Advance Article
Article type
Communication

Temperature-responsive dissolution/recrystallization of Zn MOF enables the maximum efficiency and recyclability of catalysts

X. Chen, H. Zhang, M. Zhang, Y. Zou, S. Zhang and Y. Qu, Chem. Commun., 2020, Advance Article , DOI: 10.1039/C9CC09342G

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