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Made-to-order porous electrodes for supercapacitors: MOFs embedded with redox-active centers as a case study

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Abstract

In this work, a pre-designed Zr-based-MOF encompassing an organic linker with a redox active core is synthesized and its structure–property relationship as a supercapacitor electrode is investigated. An enhanced performance is revealed by the combination of this MOF's high porosity and redox core incorporation, which alters its double-layer and pseudocapacitance, respectively. An increase in the capacitance performance by a factor of two is achieved via post-synthetic structure rigidification using organic pillars.

Graphical abstract: Made-to-order porous electrodes for supercapacitors: MOFs embedded with redox-active centers as a case study

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Article information


Submitted
13 Nov 2019
Accepted
05 Jan 2020
First published
07 Jan 2020

Chem. Commun., 2020, Advance Article
Article type
Communication

Made-to-order porous electrodes for supercapacitors: MOFs embedded with redox-active centers as a case study

A. Mallick, H. Liang, O. Shekhah, J. Jia, G. Mouchaham, A. Shkurenko, Y. Belmabkhout, H. N. Alshareef and M. Eddaoudi, Chem. Commun., 2020, Advance Article , DOI: 10.1039/C9CC08860A

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