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Issue 9, 2020
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Fine-tuning the diradical character of molecular systems via the heteroatom effect

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Abstract

Heteroatoms were introduced as a novel modification strategy for fine-tuning the diradical character of molecular systems. Both the diradical character and the singlet–triplet energy gaps of diketopyrrolopyrrole based phenoxyl diradicaloids decreased as the size of the substituted heteroatoms (from O, S to Se atom) increased.

Graphical abstract: Fine-tuning the diradical character of molecular systems via the heteroatom effect

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Article information


Submitted
01 Nov 2019
Accepted
19 Dec 2019
First published
24 Dec 2019

Chem. Commun., 2020,56, 1405-1408
Article type
Communication

Fine-tuning the diradical character of molecular systems via the heteroatom effect

W. Wang, L. Ge, G. Xue, F. Miao, P. Chen, H. Chen, Y. Lin, Y. Ni, J. Xiong, Y. Hu, J. Wu and Y. Zheng, Chem. Commun., 2020, 56, 1405
DOI: 10.1039/C9CC08538F

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