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An effective combination catalyst of CeO2 and zeolite for the direct synthesis of diethyl carbonate from CO2 and ethanol with 2,2-diethoxypropane as a dehydrating agent

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Abstract

The combination catalyst of CeO2 and H-FAU zeolite was effective for the direct synthesis of diethyl carbonate from CO2 and ethanol with 2,2-diethoxypropane as a dehydrating regent, where H-FAU catalyzed hydrolysis of 2,2-diethoxypropane. The combination catalyst provided high activity and a high diethyl carbonate yield of 72% based on 2,2-diethoxypropane at a low temperature of 393 K.

Graphical abstract: An effective combination catalyst of CeO2 and zeolite for the direct synthesis of diethyl carbonate from CO2 and ethanol with 2,2-diethoxypropane as a dehydrating agent

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Article information


Submitted
07 Aug 2020
Accepted
22 Sep 2020
First published
23 Sep 2020

Green Chem., 2020, Advance Article
Article type
Communication

An effective combination catalyst of CeO2 and zeolite for the direct synthesis of diethyl carbonate from CO2 and ethanol with 2,2-diethoxypropane as a dehydrating agent

T. Chang, M. Tamura, Y. Nakagawa, N. Fukaya, J. Choi, T. Mishima, S. Matsumoto, S. Hamura and K. Tomishige, Green Chem., 2020, Advance Article , DOI: 10.1039/D0GC02717K

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