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Issue 23, 2020
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Key factor for the anti-Arrhenius low-temperature heterogeneous catalysis induced by H+ migration: H+ coverage over support

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Abstract

Low-temperature heterogeneous catalytic reaction in an electric field is anticipated as a novel approach for on-demand and small-scale catalytic processes. This report quantitatively reveals the important role of proton coverage on the catalyst support for catalytic ammonia synthesis in an electric field, which shows an anti-Arrhenius behaviour.

Graphical abstract: Key factor for the anti-Arrhenius low-temperature heterogeneous catalysis induced by H+ migration: H+ coverage over support

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Supplementary files

Article information


Submitted
18 Jan 2020
Accepted
25 Feb 2020
First published
13 Mar 2020

This article is Open Access

Chem. Commun., 2020,56, 3365-3368
Article type
Communication

Key factor for the anti-Arrhenius low-temperature heterogeneous catalysis induced by H+ migration: H+ coverage over support

K. Murakami, Y. Tanaka, R. Sakai, Y. Hisai, S. Hayashi, Y. Mizutani, T. Higo, S. Ogo, J. G. Seo, H. Tsuneki and Y. Sekine, Chem. Commun., 2020, 56, 3365
DOI: 10.1039/D0CC00482K

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