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Photons and charges from colloidal doped semiconductor quantum dots

Abstract

The utility of colloidal semiconductor quantum dots as a source of photons and charge carriers for photonic and photovoltaic applications has created a large field of research focused on tailoring and broadening their functionality beyond what the exciton can provide. One approach towards expanding the range of characteristics of photons and charge carriers from quantum dots is through doping impurity ions (e.g. Mn2+, Cu+, and Yb3+) in the host quantum dots. In addition to the progress in the synthesis enabling the fine control of the structure of the doped quantum dots, mechanistic understanding of the underlying processes correlated with the structure has been crucial in revealing the full potential of the doped quantum dots as the source of photons and charge carriers. In this review, we discuss recent progresses made in gaining microscopic understanding of the photophysical pathways that give rise to unique dopant-related luminescence and the generation of energetic hot electrons via exciton-to-hot electron upconversion.

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Publication details

The article was received on 18 Sep 2019, accepted on 23 Oct 2019 and first published on 04 Nov 2019


Article type: Review Article
DOI: 10.1039/C9TC05150C
J. Mater. Chem. C, 2019, Accepted Manuscript

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    Photons and charges from colloidal doped semiconductor quantum dots

    T. Qiao, D. Parobek and D. H. Son, J. Mater. Chem. C, 2019, Accepted Manuscript , DOI: 10.1039/C9TC05150C

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