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Ambient Fast, Large-Scale Synthesis of Entropy-Stabilized Metal-Organic Framework Nanosheets for Electrocatalytic Oxygen Evolution

Abstract

High entropy materials, composed of the incorporation of five or more metal species into single-phase crystal structures, have received extensive attentions in many reactions. These materials achieve tailored and unexpected properties due to the interactions among various metal species. Here we report the synthesis of high entropy metal-organic framework (HE-MOF) with five near-equimolar components by solution phase method under ambient temperature. Upon served as electrocatalyst, the obtained HE-MOF performs high electrocatalytic activity toward oxygen evolution reaction in alkaline system. This strategy represents a general method to expand the library of high entropy materials and promoters for the efficient electrochemical water splitting.

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Publication details

The article was received on 09 Sep 2019, accepted on 28 Oct 2019 and first published on 28 Oct 2019


Article type: Communication
DOI: 10.1039/C9TA09975A
J. Mater. Chem. A, 2019, Accepted Manuscript

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    Ambient Fast, Large-Scale Synthesis of Entropy-Stabilized Metal-Organic Framework Nanosheets for Electrocatalytic Oxygen Evolution

    X. Zhao, Z. Xue, W. Chen, X. Bai, R. Shi and T. Mu, J. Mater. Chem. A, 2019, Accepted Manuscript , DOI: 10.1039/C9TA09975A

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