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An electron-donating strategy to guide the construction of MOF photocatalysts toward co-catalyst-free highly efficient photocatalytic H2 evolution

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Abstract

Herein, an interesting electron-donating strategy is proposed to guide the construction of novel CdS-based MOFs for co-catalyst-free photocatalytic H2 evolution in the presence of triethanolamine as the hole-scavenger. The optimally designed CdS-based MOF exhibits an exceptional H2-evolution rate of 26.1 mmol g−1 h−1 which is almost the highest rate among the reported co-catalyst-free MOF systems.

Graphical abstract: An electron-donating strategy to guide the construction of MOF photocatalysts toward co-catalyst-free highly efficient photocatalytic H2 evolution

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Publication details

The article was received on 09 Jun 2019, accepted on 15 Aug 2019 and first published on 16 Aug 2019


Article type: Communication
DOI: 10.1039/C9TA06141J
J. Mater. Chem. A, 2019, Advance Article

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    An electron-donating strategy to guide the construction of MOF photocatalysts toward co-catalyst-free highly efficient photocatalytic H2 evolution

    D. Dong, C. Yan, J. Huang, N. Lu, P. Wu, J. Wang and Z. Zhang, J. Mater. Chem. A, 2019, Advance Article , DOI: 10.1039/C9TA06141J

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