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Issue 42, 2019
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An electron-donating strategy to guide the construction of MOF photocatalysts toward co-catalyst-free highly efficient photocatalytic H2 evolution

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Abstract

Herein, an interesting electron-donating strategy is proposed to guide the construction of novel CdS-based MOFs for co-catalyst-free photocatalytic H2 evolution in the presence of triethanolamine as the hole-scavenger. The optimally designed CdS-based MOF exhibits an exceptional H2-evolution rate of 26.1 mmol g−1 h−1 which is almost the highest rate among the reported co-catalyst-free MOF systems.

Graphical abstract: An electron-donating strategy to guide the construction of MOF photocatalysts toward co-catalyst-free highly efficient photocatalytic H2 evolution

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Supplementary files

Article information


Submitted
09 Jun 2019
Accepted
15 Aug 2019
First published
16 Aug 2019

J. Mater. Chem. A, 2019,7, 24180-24185
Article type
Communication

An electron-donating strategy to guide the construction of MOF photocatalysts toward co-catalyst-free highly efficient photocatalytic H2 evolution

D. Dong, C. Yan, J. Huang, N. Lu, P. Wu, J. Wang and Z. Zhang, J. Mater. Chem. A, 2019, 7, 24180
DOI: 10.1039/C9TA06141J

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