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Ag nanoparticles with surface Cl modification (Ag–Cl NPs) by in situ electroreduction of AgCl exhibit a high selectivity for CO2-to-CO conversion. The observed C–Cl bond suggests that electrons can be effectively transferred from the Cl ions to the unoccupied orbital of CO2, and then activate nonpolar CO2 molecules on Cl sites.

Graphical abstract: Enhanced CO2 electroreduction performance over Cl-modified metal catalysts

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