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Metal–organic conjugated microporous polymer containing a carbon dioxide reduction electrocatalyst

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Abstract

A metal–organic conjugated micorporous polymer (CMP) containing a manganese carbonyl electrocatalyst for CO2 reduction has been synthesised and electrochemically characterised. Incorporation in a rigid framework changes the behavior of the catalyst, preventing reductive dimerization. These initial studies demonstrate the feasibility of CMP electrodes that can provide both high local CO2 concentrations and well defined electrocatalytic sites.

Graphical abstract: Metal–organic conjugated microporous polymer containing a carbon dioxide reduction electrocatalyst

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Publication details

The article was received on 05 Jul 2019, accepted on 08 Sep 2019 and first published on 09 Sep 2019


Article type: Communication
DOI: 10.1039/C9SE00450E
Sustainable Energy Fuels, 2019, Advance Article

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    Metal–organic conjugated microporous polymer containing a carbon dioxide reduction electrocatalyst

    C. L. Smith, R. Clowes, R. S. Sprick, A. I. Cooper and A. J. Cowan, Sustainable Energy Fuels, 2019, Advance Article , DOI: 10.1039/C9SE00450E

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