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A new redox phloroglucinol additive incorporated gel polymer electrolyte for flexible symmetrical solid-state supercapacitors

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Abstract

We reported a new and environmentally friendly phloroglucinol additive incorporated polyvinyl alcohol–LiClO4 gel polymer electrolyte for flexible symmetrical solid-state supercapacitors. The incorporation of 10 wt% phloroglucinol into PVA–LiClO4 gel polymer electrolytes results in much higher specific capacitance (114 F g−1) than that without phloroglucinol (60 F g−1), an increase of 90%, because of the redox reaction of phloroglucinol in the system. We used the PVA–LiClO4 with 10 wt% phloroglucinol as a gel polymer electrolyte in combination with nitrogen-doped graphene nanosheet-based electrodes as the anode and cathode to fabricate a symmetrical solid-state supercapacitor. The fabricated supercapacitor involving the phloroglucinol redox additive has an energy density of 2.3 W h kg−1 at a power density of 150 W kg−1, which is higher than the one without a redox additive (1.9 W h kg−1 at a power density of 150 W kg−1). Moreover, the supercapacitor involving the redox additive has good stability; its capacitance remains at up to ∼94% after 5000 charge/discharge cycles.

Graphical abstract: A new redox phloroglucinol additive incorporated gel polymer electrolyte for flexible symmetrical solid-state supercapacitors

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Publication details

The article was received on 05 Jan 2019, accepted on 11 Apr 2019 and first published on 29 Apr 2019


Article type: Paper
DOI: 10.1039/C9SE00011A
Sustainable Energy Fuels, 2019, Advance Article

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    A new redox phloroglucinol additive incorporated gel polymer electrolyte for flexible symmetrical solid-state supercapacitors

    P. Le, V. Nguyen, P. Yen, T. Tseng and K. Wei, Sustainable Energy Fuels, 2019, Advance Article , DOI: 10.1039/C9SE00011A

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