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Synthesis of novel bimetallic nickel cobalt telluride nanotubes on nickel foam for high-performance hybrid supercapacitors

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Abstract

To improve the energy density of a supercapacitor while maintaining its high power density, novel bimetallic nickel cobalt telluride nanotubes are synthesized on nickel foam by a facile solvothermal synthesis followed by an ion-exchange reaction for constructing self-standing hybrid supercapacitor electrodes with high specific capacity and electrical conductivity. The nickel cobalt nanosheets generated by solvothermal synthesis are converted to nickel cobalt telluride nanotubes during the ion-exchange reaction process in the presence of Na2TeO3 at 180 °C. The resultant Ni0.33Co0.67Te nanotubes with large aspect ratios and thin walls form a robust interpenetrating network on nickel foam, providing convenient ion/electron transport channels and accessible contact of the electrode with electrolyte. Benefiting from such a nanotubular structure, the Ni0.33Co0.67Te nanotube electrode delivers a high specific capacity of 131.2 mA h g−1 at 1 A g−1 and 79.3 mA h g−1 at 20 A g−1 with satisfactory cycling durability. Furthermore, the assembled Ni0.33Co0.67Te nanotube//active carbon hybrid supercapacitor achieves a high energy density of 54.0 W h kg−1 at a power density of 918 W kg−1, and a long-term cycling stability with 90% of capacity retention after 5000 cycles. This work provides a simple and efficient approach to produce bimetallic nickel cobalt telluride nanotube electrodes for high-performance hybrid supercapacitors.

Graphical abstract: Synthesis of novel bimetallic nickel cobalt telluride nanotubes on nickel foam for high-performance hybrid supercapacitors

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Publication details

The article was received on 27 Oct 2019, accepted on 06 Nov 2019 and first published on 06 Nov 2019


Article type: Research Article
DOI: 10.1039/C9QI01395D
Inorg. Chem. Front., 2019, Advance Article

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    Synthesis of novel bimetallic nickel cobalt telluride nanotubes on nickel foam for high-performance hybrid supercapacitors

    S. Zhang, D. Yang, M. Zhang, Y. Liu, T. Xu, J. Yang and Z. Yu, Inorg. Chem. Front., 2019, Advance Article , DOI: 10.1039/C9QI01395D

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