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Solid-state-stabilization of molecular vanadium oxides for reversible electrochemical charge storage

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Abstract

Molecular vanadium oxides are promising active materials for cathodes in lithium and post-lithium batteries due to their high redox activity, low molecular weight and facile tuneability. However, a major challenge for this application is the transformation of the molecular clusters into solid-state oxides under typical electrode fabrication conditions. Here, we report a molecular crystal engineering approach for the stabilization of molecular vanadium oxides in the crystal lattice, enabling initial studies on reversible electron storage in a lithium ion battery test cell.

Graphical abstract: Solid-state-stabilization of molecular vanadium oxides for reversible electrochemical charge storage

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Publication details

The article was received on 24 Sep 2019, accepted on 23 Oct 2019 and first published on 24 Oct 2019


Article type: Research Article
DOI: 10.1039/C9QI01229J
Inorg. Chem. Front., 2019, Advance Article

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    Solid-state-stabilization of molecular vanadium oxides for reversible electrochemical charge storage

    S. Greiner, M. H. Anjass, M. Fichtner and C. Streb, Inorg. Chem. Front., 2019, Advance Article , DOI: 10.1039/C9QI01229J

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