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BaMnSnS4 and BaCdGeS4: infrared nonlinear optical sulfides containing highly distorted motifs with centers of moderate electronegativity

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Abstract

IR NLO sulfides BaMnSnS4 and BaCdGeS4 exhibit significant SHG efficiencies (1.2 and 0.3AgGaS2) with phase-matching behavior and high laser-induced damage thresholds (10 and 13AgGaS2). Their strong SHG efficiencies mainly originate from SnS4 and GeS4 tetrahedra that are being modulated by highly distorted MnS4 and CdS4 tetrahedra.

Graphical abstract: BaMnSnS4 and BaCdGeS4: infrared nonlinear optical sulfides containing highly distorted motifs with centers of moderate electronegativity

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Publication details

The article was received on 17 Jun 2019, accepted on 17 Jul 2019 and first published on 19 Jul 2019


Article type: Research Article
DOI: 10.1039/C9QI00727J
Inorg. Chem. Front., 2019, Advance Article

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    BaMnSnS4 and BaCdGeS4: infrared nonlinear optical sulfides containing highly distorted motifs with centers of moderate electronegativity

    Y. Lin, R. Ye, L. Yang, X. Jiang, B. Liu, H. Zeng and G. Guo, Inorg. Chem. Front., 2019, Advance Article , DOI: 10.1039/C9QI00727J

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