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Issue 39, 2019
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Facile access to evodiakine enabled by aerobic copper-catalyzed oxidative rearrangement

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Abstract

Oxidation as a fundamentally important method for the synthesis of complex structures is difficult to achieve in a selective manner. Evodiakine, a complex natural product possessing an unprecedented ring system (6/5/5/7/6), has a high oxidation state without a practical solution. Herein, we report the first synthesis of evodiakine via aerobic copper-catalyzed late-stage functionalization of evodiamine.

Graphical abstract: Facile access to evodiakine enabled by aerobic copper-catalyzed oxidative rearrangement

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Publication details

The article was received on 20 Aug 2019, accepted on 24 Sep 2019 and first published on 25 Sep 2019


Article type: Communication
DOI: 10.1039/C9OB01832H
Org. Biomol. Chem., 2019,17, 8811-8815

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    Facile access to evodiakine enabled by aerobic copper-catalyzed oxidative rearrangement

    Y. Su, G. Huang, F. Ye, P. Qiao, J. Ye, Y. Gao and H. Chen, Org. Biomol. Chem., 2019, 17, 8811
    DOI: 10.1039/C9OB01832H

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