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Issue 7, 2019
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Synthesis of the core structure of phalarine

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Abstract

The core skeleton of phalarine was rapidly synthesised through novel palladium-catalysed dearomative spirocyclisation and a palladium-catalysed Wacker-carbonylative cyclisation cascade. The two key steps allowed for the efficient construction of a tricyclic propeller skeleton bearing contiguous tetrasubstituted carbon centres, within 3 steps from a topologically planar precursor.

Graphical abstract: Synthesis of the core structure of phalarine

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Supplementary files

Article information


Submitted
19 Sep 2018
Accepted
29 Sep 2018
First published
01 Oct 2018

Org. Biomol. Chem., 2019,17, 1727-1730
Article type
Communication
Author version available

Synthesis of the core structure of phalarine

K. Douki, J. Shimokawa and M. Kitamura, Org. Biomol. Chem., 2019, 17, 1727
DOI: 10.1039/C8OB02320D

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