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Superior phototransistors based on a single ZnO nanoparticle with high mobility and ultrafast response time

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Abstract

Conventional film-structured polycrystalline semiconductor devices suffer from grain boundary scattering, which is responsible for low mobility and can even mask intrinsic transport properties. In this work, we show that devices containing only a ZnO single particle can exhibit mobility values one order higher than that of single-crystal nanowires. The ZnO nanoparticle was embedded inside a nanopore structure, surrounded by a gate electrode and connected to top and bottom electrodes. Due to the absence of inter-grain scattering and long traveling distance, we obtained relatively high mobility values of around 600 cm2 V−1 s−1 at room temperature (300 K) and about 1100 cm2 V−1 s−1 at low temperature (∼180 K). The devices also presented external quantum efficiency of 5.6 × 107, responsivity of 1.39 × 106 AW−1, detectivity of 8.69 × 1012 Jones, and a record-high photoresponse rise time of 90 μs. This single nanoparticle-based device could be an excellent candidate of phototransistors with high performances.

Graphical abstract: Superior phototransistors based on a single ZnO nanoparticle with high mobility and ultrafast response time

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Publication details

The article was received on 08 May 2019, accepted on 07 Aug 2019 and first published on 07 Aug 2019


Article type: Communication
DOI: 10.1039/C9NH00299E
Nanoscale Horiz., 2019, Advance Article

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    Superior phototransistors based on a single ZnO nanoparticle with high mobility and ultrafast response time

    L. Nguyen, W. Chang, C. Chen and Y. Lan, Nanoscale Horiz., 2019, Advance Article , DOI: 10.1039/C9NH00299E

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