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Morphology control in semicrystalline solid polymer electrolytes for lithium batteries

Abstract

Solid polymer electrolytes (SPEs) are one of the most promising solutions to the safety issues of lithium batteries. Understanding the morphology and dynamic effects on the ion transport properties of SPEs would be essential for future SPE design. In this article, using Poly(ethylene oxide) (PEO) as the example, we will discuss the morphology control in semicrystalline SPEs. We show that the effect of semicrystallinity can be quantitatively separated into volume, structure and dynamic effects. We further demonstrate that morphological control plays an important role in ion transport control in semicrystalline SPE systems.

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Publication details

The article was received on 21 Feb 2019, accepted on 16 May 2019 and first published on 16 May 2019


Article type: Perspective
DOI: 10.1039/C9ME00028C
Mol. Syst. Des. Eng., 2019, Accepted Manuscript

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    Morphology control in semicrystalline solid polymer electrolytes for lithium batteries

    X. Li, S. Cheng, Y. Zheng and C. Li, Mol. Syst. Des. Eng., 2019, Accepted Manuscript , DOI: 10.1039/C9ME00028C

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