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Cobalt-catalyzed alkylation of methyl-substituted N-heteroarenes with primary alcohols: direct access to functionalized N-heteroaromatics

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Abstract

Phosphine free, air and moisture stable Co(NNN) complex catalyzed alkylation of various methyl-substituted N-heteroarenes with alcohols is reported. Following the borrowing hydrogen methodology, a variety of methyl-substituted N-heteroarenes can be functionalized efficiently. To understand the mechanism of this reaction various kinetic and control experiments were carried out.

Graphical abstract: Cobalt-catalyzed alkylation of methyl-substituted N-heteroarenes with primary alcohols: direct access to functionalized N-heteroaromatics

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Publication details

The article was received on 29 Oct 2019, accepted on 27 Nov 2019 and first published on 27 Nov 2019


Article type: Communication
DOI: 10.1039/C9CC08448G
Chem. Commun., 2020, Advance Article

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    Cobalt-catalyzed alkylation of methyl-substituted N-heteroarenes with primary alcohols: direct access to functionalized N-heteroaromatics

    A. Mishra, A. D. Dwivedi, S. Shee and S. Kundu, Chem. Commun., 2020, Advance Article , DOI: 10.1039/C9CC08448G

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