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A tri-functional metal–organic framework heterogeneous catalyst for efficient conversion of CO2 under mild and co-catalyst free conditions

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Abstract

Herein, we developed a tri-functional MOF heterogeneous catalyst, MIL-IMAc-Br, by a post-synthesis modification method for the first time. Due to the synergistic role of three functional sites, including Lewis acid sites, Brønsted acid sites and Br anion sites, MIL-IMAc-Br displayed an efficient catalytic performance for the cycloaddition reaction of CO2 and epoxides to form cyclic carbonates under mild and co-catalyst free conditions.

Graphical abstract: A tri-functional metal–organic framework heterogeneous catalyst for efficient conversion of CO2 under mild and co-catalyst free conditions

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Publication details

The article was received on 21 Oct 2019, accepted on 04 Nov 2019 and first published on 05 Nov 2019


Article type: Communication
DOI: 10.1039/C9CC08236K
Chem. Commun., 2019, Advance Article

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    A tri-functional metal–organic framework heterogeneous catalyst for efficient conversion of CO2 under mild and co-catalyst free conditions

    D. Ma, Y. Zhang, S. Jiao, J. Li, K. Liu and Z. Shi, Chem. Commun., 2019, Advance Article , DOI: 10.1039/C9CC08236K

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