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A robust photocatalyst of Au25@ZIF-8@TiO2-ReP with dual photoreductive sites to promote photoelectron utilization in H2O splitting to H2 and CO2 reduction to CO

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Abstract

Sustaining long-term chemical or photochemical stability of a homogeneous molecular catalyst remains a significant challenge. We report a remarkable improvement of the activity and stability of a Au25@ZIF-8@TiO2-ReP catalyst via composition engineering with double redox active sites of Au25 NCs and a Re(I) complex for H2 and CO evolution to promote electron utilization.

Graphical abstract: A robust photocatalyst of Au25@ZIF-8@TiO2-ReP with dual photoreductive sites to promote photoelectron utilization in H2O splitting to H2 and CO2 reduction to CO

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Publication details

The article was received on 10 Sep 2019, accepted on 03 Oct 2019 and first published on 04 Oct 2019


Article type: Communication
DOI: 10.1039/C9CC07014A
Chem. Commun., 2019, Advance Article

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    A robust photocatalyst of Au25@ZIF-8@TiO2-ReP with dual photoreductive sites to promote photoelectron utilization in H2O splitting to H2 and CO2 reduction to CO

    L. Tian, Y. Luo, K. Chu, D. Wu, J. Shi and Z. Liang, Chem. Commun., 2019, Advance Article , DOI: 10.1039/C9CC07014A

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