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Issue 91, 2019
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Synergistic photothermal and photochemical partial oxidation of methane over noble metals incorporated in mesoporous silica

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Abstract

A hot-carrier-driven photocatalytic system was established by incorporating noble metals (Rh, Pd, Ru, and Pt) in a mesoporous silica (MCM-41) for the partial oxidation of methane (POM) under ultraviolet (UV) irradiation. The Rh/MCM photocatalyst initiated POM at a mild operating temperature of 423 K with syngas generation. The reaction was identified as a synergistic photothermal and photochemical process.

Graphical abstract: Synergistic photothermal and photochemical partial oxidation of methane over noble metals incorporated in mesoporous silica

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Publication details

The article was received on 09 Aug 2019, accepted on 22 Oct 2019 and first published on 22 Oct 2019


Article type: Communication
DOI: 10.1039/C9CC06170C
Chem. Commun., 2019,55, 13765-13768

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    Synergistic photothermal and photochemical partial oxidation of methane over noble metals incorporated in mesoporous silica

    H. Jiang, X. Peng, A. Yamaguchi, T. Fujita, H. Abe and M. Miyauchi, Chem. Commun., 2019, 55, 13765
    DOI: 10.1039/C9CC06170C

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