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Silane catecholates: versatile tools for self-assembled dynamic covalent bond chemistry

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Abstract

Shape-persistent macrocycles and 3D nanocages have been prepared in one-pot under MeCN-promoted dynamic covalent bond conditions starting from silane catecholates, whose structures were confirmed by X-ray crystallography. Cation-exchange reactions of macrocycles and nanocages were performed along with the encapsulation of ammonium ions within the cavity of an anionic macrocycle and a tetrahedral nanocage.

Graphical abstract: Silane catecholates: versatile tools for self-assembled dynamic covalent bond chemistry

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Publication details

The article was received on 15 Mar 2019, accepted on 27 Apr 2019 and first published on 29 Apr 2019


Article type: Communication
DOI: 10.1039/C9CC02103E
Chem. Commun., 2019, Advance Article

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    Silane catecholates: versatile tools for self-assembled dynamic covalent bond chemistry

    Y. Kawakami, T. Ogishima, T. Kawara, S. Yamauchi, K. Okamoto, S. Nikaido, D. Souma, R. Jin and Y. Kabe, Chem. Commun., 2019, Advance Article , DOI: 10.1039/C9CC02103E

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