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Elucidating the mechanism of the structure-dependent enzymatic activity of Fe–N/C oxidase mimics

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Abstract

Herein, we develop an Fe–N/C–CNT nanomaterial with Fe–N3 units as a paradigm for excellent oxidase mimics by theoretical prediction and experimental implementation. The mechanism of the structure-dependent enzymatic activity is systematically investigated and elucidated from the perspective of the different configurations of M–Nx models (x = 0, 3, 4, and 5; M = Fe, Co, and Ni).

Graphical abstract: Elucidating the mechanism of the structure-dependent enzymatic activity of Fe–N/C oxidase mimics

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Publication details

The article was received on 21 Feb 2019, accepted on 11 Apr 2019 and first published on 11 Apr 2019


Article type: Communication
DOI: 10.1039/C9CC01503E
Citation: Chem. Commun., 2019, Advance Article

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    Elucidating the mechanism of the structure-dependent enzymatic activity of Fe–N/C oxidase mimics

    Y. Wang, Z. Zhang, G. Jia, L. Zheng, J. Zhao and X. Cui, Chem. Commun., 2019, Advance Article , DOI: 10.1039/C9CC01503E

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