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Issue 39, 2019
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Optimizing electron transfer from CdSe QDs to hydrogenase for photocatalytic H2 production

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Abstract

A series of viologen related redox mediators of varying reduction potential has been characterized and their utility as electron shuttles between CdSe quantum dots and hydrogenase enzyme has been demonstrated. Tuning the mediator LUMO energy optimizes the performance of this hybrid photocatalytic system by balancing electron transfer rates of the shuttle.

Graphical abstract: Optimizing electron transfer from CdSe QDs to hydrogenase for photocatalytic H2 production

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Article information


Submitted
08 Feb 2019
Accepted
11 Apr 2019
First published
11 Apr 2019

Chem. Commun., 2019,55, 5579-5582
Article type
Communication
Author version available

Optimizing electron transfer from CdSe QDs to hydrogenase for photocatalytic H2 production

M. L. K. Sanchez, C. Wu, M. W. W. Adams and R. B. Dyer, Chem. Commun., 2019, 55, 5579
DOI: 10.1039/C9CC01150A

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