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Supramolecular aggregation of a redox-active copper-naphthalenediimide network with intrinsic electron conduction

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Abstract

A sextuple ordered interpenetrated copper-naphthalenediimide network has been constructed by combining the features of porous metal–organic frameworks and π-conjugated supramolecular aggregation. The material exhibits intrinsic semiconductive features with narrow bandgap energy (1.2 eV) and outstanding electron transport. Theoretical calculations combined with experiments indicate that the high electron conduction may originate from π–d coupling and J-aggregation.

Graphical abstract: Supramolecular aggregation of a redox-active copper-naphthalenediimide network with intrinsic electron conduction

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Publication details

The article was received on 29 Dec 2018, accepted on 11 Jan 2019 and first published on 12 Jan 2019


Article type: Communication
DOI: 10.1039/C8CC10269D
Citation: Chem. Commun., 2019, Advance Article
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    Supramolecular aggregation of a redox-active copper-naphthalenediimide network with intrinsic electron conduction

    X. Kuang, S. Chen, L. Meng, J. Chen, X. Wu, G. Zhang, G. Zhong, T. Hu, Y. Li and C. Lu, Chem. Commun., 2019, Advance Article , DOI: 10.1039/C8CC10269D

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