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Leachate emissions of short- and long-chain per- and polyfluoralkyl substances (PFASs) from various Norwegian landfills

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Abstract

Restrictions on the use of long-chain per- and polyfluoralkyl substances (PFASs) has led to substitutions with short-chain PFASs. This study investigated the presence of four short-chain PFASs and twenty-four long-chain PFASs in leachate and sediment from ten Norwegian landfills, including one site in Svalbard, to assess whether short-chain PFASs are more dominant in leachate. PFASs were detected in all sites. Short-chain PFASs were major contributors to the total PFAS leachate concentrations in six of ten landfills, though not in Svalbard. In sediment, long-chain PFASs such as perfluorooctanesulfonate (PFOS) and PFOS-precursors were dominant. Short-chain PFAS leachate concentrations ranged from 68 to 6800 ng L−1 (mean: 980 ± 1800; median: 360 ng L−1), whereas long-chain concentrations ranged from 140 to 2900 ng L−1 (mean: 530 ± 730; median: 290 ng L−1). Sediment concentrations, which contained mainly long-chain PFASs, ranged from 8.5 to 120 μg kg−1 (mean: 47 ± 36; median: 41 μg kg−1). National Image ID:c9em00170k-t1.gif release from Norwegian landfills to the environment was estimated to be 17 ± 29 kg per year (median: 6.3 kg per year), which is in the same range as national emissions from the US, China and Germany after normalizing the data to a per capita emission factor (3.2 ± 5.5 mg per person per year). Results from this study are compared with previous and current studies in other countries, indicating a general trend that short-chain PFASs are dominating over long-chain PFASs in landfill leachate emissions.

Graphical abstract: Leachate emissions of short- and long-chain per- and polyfluoralkyl substances (PFASs) from various Norwegian landfills

  • This article is part of the themed collection: PFAS
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Publication details

The article was received on 10 Apr 2019, accepted on 07 Aug 2019 and first published on 09 Aug 2019


Article type: Paper
DOI: 10.1039/C9EM00170K
Environ. Sci.: Processes Impacts, 2019, Advance Article
  • Open access: Creative Commons BY license
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    Leachate emissions of short- and long-chain per- and polyfluoralkyl substances (PFASs) from various Norwegian landfills

    H. Knutsen, T. Mæhlum, K. Haarstad, G. A. Slinde and H. P. H. Arp, Environ. Sci.: Processes Impacts, 2019, Advance Article , DOI: 10.1039/C9EM00170K

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