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Issue 14, 2019
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Homogeneously-catalysed hydrogen release/storage using the 2-methylindole/2-methylindoline LOHC system in molten salt-organic biphasic reaction systems

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Abstract

Ir-Complex catalysed hydrogen release/storage using a 2-methylindole/2-methylindoline Liquid Organic Hydrogen Carrier (LOHC) system is shown to be effective in a temperature range of 120 to 140 °C. In the form of a liquid–liquid biphasic reaction system with molten [PPh4][NTf2] as catalyst immobilisation phase, the applied cationic Ir-complex can be easily separated and recycled enabling a small amount of ionic catalyst solution to store/release a large amount of hydrogen.

Graphical abstract: Homogeneously-catalysed hydrogen release/storage using the 2-methylindole/2-methylindoline LOHC system in molten salt-organic biphasic reaction systems

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Article information


Submitted
13 Dec 2018
Accepted
18 Jan 2019
First published
18 Jan 2019

Chem. Commun., 2019,55, 2046-2049
Article type
Communication

Homogeneously-catalysed hydrogen release/storage using the 2-methylindole/2-methylindoline LOHC system in molten salt-organic biphasic reaction systems

A. Søgaard, M. Scheuermeyer, A. Bösmann, P. Wasserscheid and A. Riisager, Chem. Commun., 2019, 55, 2046
DOI: 10.1039/C8CC09883B

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