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Issue 36, 2018
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Illuminating the nature and behavior of the active center: the key for photocatalytic H2 production in Co@NH2-MIL-125(Ti)

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Abstract

Advanced atomically resolved characterization methods unveil the mechanism of a promising photocatalytic Co@MOF(Ti) system for H2 production. The combination of X-ray absorption spectroscopy (XAS) and electron paramagnetic resonance (EPR) experiments allows for the characterization of atomic and electronic rearrangements in the photoinduced species. This information provides the basis for the optimization of photocatalyst design.

Graphical abstract: Illuminating the nature and behavior of the active center: the key for photocatalytic H2 production in Co@NH2-MIL-125(Ti)

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Supplementary files

Article information


Submitted
15 Jun 2018
Accepted
16 Aug 2018
First published
22 Aug 2018

J. Mater. Chem. A, 2018,6, 17318-17322
Article type
Communication

Illuminating the nature and behavior of the active center: the key for photocatalytic H2 production in Co@NH2-MIL-125(Ti)

A. Iglesias-Juez, S. Castellanos, M. Monte, G. Agostini, D. Osadchii, M. A. Nasalevich, J. G. Santaclara, A. I. Olivos Suarez, S. L. Veber, M. V. Fedin and J. Gascón, J. Mater. Chem. A, 2018, 6, 17318
DOI: 10.1039/C8TA05735D

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