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Continuous flow aerobic alcohol oxidation using a heterogeneous Ru0 catalyst

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Abstract

The continuous selective aerobic oxidation of benzyl alcohol in flow was developed using an immobilized Ru0 catalyst. After optimization of the reaction conditions, the stability and productivity of the equipment were examined over time using tert-amyl alcohol as solvent, and no deactivation occurred. A cumulative TON close to 15 000 was obtained with a constant activity (TOF = 4 min−1). A semi-empirical kinetic rate expression was proposed.

Graphical abstract: Continuous flow aerobic alcohol oxidation using a heterogeneous Ru0 catalyst

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Publication details

The article was received on 25 Sep 2018, accepted on 29 Nov 2018 and first published on 30 Nov 2018


Article type: Paper
DOI: 10.1039/C8RE00212F
Citation: React. Chem. Eng., 2019, Advance Article
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    Continuous flow aerobic alcohol oxidation using a heterogeneous Ru0 catalyst

    J. Sofack Kreutzer, L. Vanoye, B. Guicheret, R. Philippe, E. Metay, M. Duclos, M. Lemaire, C. De Bellefon, P. Fongarland and A. Favre-Réguillon, React. Chem. Eng., 2019, Advance Article , DOI: 10.1039/C8RE00212F

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