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Issue 21, 2018
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Visible-light initiated aerobic oxidations: a critical review

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The development of new and highly efficient strategies for the rapid construction of complicated molecular structures has huge implications and remains a preeminent goal in present day synthetic chemistry. In the past ten years, visible light promoted aerobic oxidations have been emerging as one of the fastest growing fields in organic chemistry because of their low cost, easy availability and environmental friendliness. This review describes and highlights the scope and limitations, recent research progress in novel methodology development, and applications in organic synthesis, as well as the mechanisms of these visible light promoted aerobic oxidation reactions. The discussion contains several sections based on the following reaction types: (1) alcohols to aldehydes; (2) amines to nitriles; (3) methylarenes to aldehydes; (4) boronic acids to phenols; (5) formation of carbonyl compounds or ketones; (6) β-keto sulfones; (7) sulfoxides; (8) amine to amide; and (9) some other reactions.

Graphical abstract: Visible-light initiated aerobic oxidations: a critical review

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Publication details

The article was received on 30 Jul 2018, accepted on 21 Sep 2018 and first published on 08 Oct 2018

Article type: Critical Review
DOI: 10.1039/C8GC02382D
Green Chem., 2018,20, 4790-4833

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    Visible-light initiated aerobic oxidations: a critical review

    X. Zhang, K. P. Rakesh, L. Ravindar and H. Qin, Green Chem., 2018, 20, 4790
    DOI: 10.1039/C8GC02382D

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