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Thermal-exfoliated synthesis of N-rich carbon-based nanosheets from layered bulk crystals of a metal–hexamine framework

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Abstract

We develop a general strategy for the design of a series of 2D N-rich carbon-based nanomaterials through the thermal exfoliation of layered metal–hexamine framework microcrystals. By a facile pyrolysis, the sharply generated gases escape from the layered precursors, leading to the exfoliation of the layers and successful preparation of 2D carbon-based nanomaterials. This strategy can readily skip the complicated morphology engineering process of 2D metal–organic frameworks to produce 2D N-rich carbon-based nanomaterials on a large scale.

Graphical abstract: Thermal-exfoliated synthesis of N-rich carbon-based nanosheets from layered bulk crystals of a metal–hexamine framework

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Publication details

The article was received on 22 Jun 2018, accepted on 03 Aug 2018 and first published on 06 Aug 2018


Article type: Communication
DOI: 10.1039/C8CC04988B
Citation: Chem. Commun., 2018, Advance Article
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    Thermal-exfoliated synthesis of N-rich carbon-based nanosheets from layered bulk crystals of a metal–hexamine framework

    S. Liu, J. Zhou and H. Song, Chem. Commun., 2018, Advance Article , DOI: 10.1039/C8CC04988B

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