Dynamic time-resolved Raman spectroelectrochemistry demonstrates the strong influence of nanostructuring and surface charge of in situ activated disposable substrates for SERS detection. Under specific conditions, a large enhancement factor and estimated calculations agree with the feasible detection of only a few molecules, approaching the limit of single-entity detection.
D. Martín-Yerga, A. Pérez-Junquera, M. B. González-García, D. Hernández-Santos and P. Fanjul-Bolado, Chem. Commun., 2018, 54, 5748 DOI: 10.1039/C8CC02069H
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