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Issue 27, 2018
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Optimization of energy transfer in a polymer composite with perylene chromophores

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Abstract

Luminescent solar concentrators based on molecular dyes are a promising approach to light collection for photovoltaics owing to their potential low cost and wide light acceptance angles. However, they readily suffer from self-absorption, which rapidly reduces device efficiency. We use a perylene-based sensitizer–emitter system to reduce self-absorption. The sensitizer and emitter are copolymerized to enhance energy transfer to the emitter. The sensitizer is susceptible to yield-reducing H-aggregation. We show that a composite polymer can be used to reduce H-aggregation, while maintaining efficient energy transfer.

Graphical abstract: Optimization of energy transfer in a polymer composite with perylene chromophores

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Publication details

The article was received on 21 May 2018, accepted on 19 Jun 2018 and first published on 29 Jun 2018


Article type: Paper
DOI: 10.1039/C8TC02457J
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J. Mater. Chem. C, 2018,6, 7333-7342

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    Optimization of energy transfer in a polymer composite with perylene chromophores

    V. B. Yasarapudi, L. Frazer, N. J. L. K. Davis, E. P. Booker, A. Macmillan, J. K. Gallaher, D. Roberts, S. Perrier and T. W. Schmidt, J. Mater. Chem. C, 2018, 6, 7333
    DOI: 10.1039/C8TC02457J

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