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Issue 10, 2017
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Vapor-fed solar hydrogen production exceeding 15% efficiency using earth abundant catalysts and anion exchange membrane

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Abstract

Vapor-fed solar hydrogen generators can convert water vapor from the air into hydrogen using sunlight as the energy source. Hydrogen and oxygen evolution reactions are performed in the gas phase in cathode and anode compartments separated by a membrane. Anion exchange membranes show great promise for this type of solar hydrogen generator. They provide an alkaline environment enabling the use of earth abundant materials as electrocatalysts. In this work, a vapor-fed solar hydrogen generator with KOH-doped poly(vinyl alcohol) anion exchange membrane flanked with NiFe and NiMo catalysts is demonstrated. The device reached an average 15.1% solar-to-hydrogen efficiency at room temperature and 95% relative humidity. This first demonstration of gas phase water splitting with earth abundant catalysts and anion exchange membrane opens a pathway to low cost, autonomous, efficient and safe solar hydrogen generators.

Graphical abstract: Vapor-fed solar hydrogen production exceeding 15% efficiency using earth abundant catalysts and anion exchange membrane

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Article information


Submitted
02 Aug 2017
Accepted
24 Sep 2017
First published
25 Sep 2017

Sustainable Energy Fuels, 2017,1, 2061-2065
Article type
Communication

Vapor-fed solar hydrogen production exceeding 15% efficiency using earth abundant catalysts and anion exchange membrane

G. Heremans, C. Trompoukis, N. Daems, T. Bosserez, I. F. J. Vankelecom, J. A. Martens and J. Rongé, Sustainable Energy Fuels, 2017, 1, 2061
DOI: 10.1039/C7SE00373K

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