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Issue 28, 2017
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1,2-Difunctionalization-type (hetero)arylation of unactivated alkenes triggered by radical addition/remote (hetero)aryl migration

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Abstract

A novel difunctionalization-type (hetero)arylation of unactivated alkenes has been developed via remote 1,4(5)-(hetero)aryl migration triggered by radical alkene azidation, trifluoromethylation, or phosphonylation. The overall process serves as an unusual and reliable approach for straightforward access to diversely substituted ketones with broad functional group compatibility from readily available substrates and reagents.

Graphical abstract: 1,2-Difunctionalization-type (hetero)arylation of unactivated alkenes triggered by radical addition/remote (hetero)aryl migration

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Article information


Submitted
18 Nov 2016
Accepted
13 Mar 2017
First published
15 Mar 2017

Chem. Commun., 2017,53, 4038-4041
Article type
Communication

1,2-Difunctionalization-type (hetero)arylation of unactivated alkenes triggered by radical addition/remote (hetero)aryl migration

L. Li, Q. Gu, N. Wang, P. Song, Z. Li, X. Li, F. Wang and X. Liu, Chem. Commun., 2017, 53, 4038
DOI: 10.1039/C6CC09215B

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