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Abstract | Cited by

Here, we report the first X-ray crystal structure of a tetrathiafulvalene-fused dehydroannulene with peripheral ethylthio substituents. In addition, we have subjected this compound to electrochemical and UV-Vis-NIR/ESR spectroelectrochemical studies to elucidate the degree to which the oxidised species associate.

Graphical abstract: On the association of neutral and cationic tris(tetrathiafulvaleno)dodecadehydro[18]annulenes

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